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I will discuss our efforts on the synthesis, stability, and catalytic activity of OICs prepared by electrochemical methods at room temperature and atmospheric pressure. Our strategies include the use of electrochemically induced phase transformations which enables us to convert a base metal rich alloy to an OIC richer in nobler metal by removal of the base metal, and the direct production of OIC materials by electrochemical deposition. We will also discuss how we leverage the atomically precise configuration of atoms within OICs to reveal detailed insights into how a material\u00e2\u0080\u0099s structure regulates its electrochemical properties. 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